Burnout of soot particles in a two-stage burner with a JP-8 surrogate fuel

Carlos A. Echavarria, Isabel C. Jaramillo, Adel F. Sarofim, Jo Ann S. Lighty

Research output: Contribution to journalArticlepeer-review

64 Scopus citations

Abstract

This work focuses on the understanding of the oxidation of soot particles which were the result of using a JP-8 surrogate fuel in a two-stage burner. The two-stage system consists of an initial premixed burner where soot was generated with an air/fuel mixture, specifically a JP-8 surrogate (m-xylene and n-dodecane), under a variety of conditions. Downstream, the soot-laden combustion gases were passed through a second, flat-flame burner where soot was burned out under fuel-lean or slightly fuel-rich conditions. Soot oxidation in the secondary burner was determined by investigating particle size distribution (PSD), flame temperature, gas-phase composition, soot surface area, and soot morphology and nanostructure as a function of the height above the second burner (HAB). Measurements of soot size distribution and number concentration as a function of the HAB under fuel lean (Φoverall=0.8) and slightly rich (Φoverall=1.14) conditions showed a decrease in particle mean diameter and a significant increase in number concentration in the region where O 2 concentration decreased. In this region, the effectiveness factor for O 2 was found to be 1, indicating the potential for internal oxygen diffusion and burning. This caused both the breakup of the bridges cementing primary particles and the rupture of the primary particles. Higher in the burner, where modeling suggested the presence of OH *, soot oxidation was attributed to OH * mechanisms which are faster as compared to O 2 oxidation.

Original languageEnglish
Pages (from-to)2441-2448
Number of pages8
JournalCombustion and Flame
Volume159
Issue number7
DOIs
StatePublished - Jul 2012

Keywords

  • JP-8
  • M-Xylene flames
  • N-Dodecane flames
  • Soot oxidation
  • Soot size distribution

EGS Disciplines

  • Chemical Engineering

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