Multidimensional coherent spectroscopy made easy

Kenan Gundogdu; Katherine W. Stone; Daniel B. Turner; Keith A. Nelson

doi:10.1016/j.chemphys.2007.06.027

Multidimensional coherent spectroscopy made easy

Kenan Gundogdu, Katherine W. Stone, Daniel B. Turner, Keith A. Nelson

Massachusetts Institute of Technology

Research output: Contribution to journal › Article › peer-review

62 Scopus citations

Abstract

We have demonstrated a highly efficient fully coherent 2D spectrometer based on 2D pulse shaping and Fourier beam shaping. The versatility of the design allows one to measure different 2D spectral surfaces consecutively. Easy alignment, inherent phase stability, rotating wave frame detection, and arbitrary waveform generation in all of the beams are important features of this design. We have demonstrated the functionality of the 2D spectrometer by measuring a 2D spectral surface of a GaAs quantum well.

Original language	English
Pages (from-to)	89-94
Number of pages	6
Journal	Chemical Physics
Volume	341
Issue number	1-3
DOIs	https://doi.org/10.1016/j.chemphys.2007.06.027
State	Published - 15 Nov 2007
Externally published	Yes

Keywords

Coherent
Four-wave mixing
Multidimensional spectroscopy
Pulse shaping
Ultrafast spectroscopy

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10.1016/j.chemphys.2007.06.027

Cite this

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keywords = "Coherent, Four-wave mixing, Multidimensional spectroscopy, Pulse shaping, Ultrafast spectroscopy",

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AU - Turner, Daniel B.

AU - Nelson, Keith A.

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KW - Coherent

KW - Four-wave mixing

KW - Multidimensional spectroscopy

KW - Pulse shaping

KW - Ultrafast spectroscopy

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DO - 10.1016/j.chemphys.2007.06.027

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EP - 94

JO - Chemical Physics

JF - Chemical Physics

IS - 1-3

ER -

Multidimensional coherent spectroscopy made easy

Abstract

Keywords

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